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    Development of N-heterocyclic carbenes for application in the intermolecular stetter reaction, The

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    http://hdl.handle.net/10217/67900
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    Abstract
    An N-heterocyclic carbene scaffold has been developed containing a protected oxygen moiety in the backbone. The oxygen provides a similar electronic effect known to fluorinated analogues, and also has the potential to be modulated via substitution. This substitution introduces steric differentiation distil to the reaction site and electronic manipulation of the calculated catalyst substrate interaction. A short synthesis has been designed with an intermediate that allows for divergent manipulation of the oxygen substituent. The resultant carbenes catalyze the intermolecular Stetter reaction with ...
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    Author(s)
    Rhorer, Timothy Benjamin

    Advisor(s)
    Rovis, Tomislav

    Date Issued
    2012
    Format
    born digital; masters theses
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    • 2000-2019 - CSU Theses and Dissertations
    • Theses and Dissertations - Department of Chemistry

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