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²²⁶Ra contamination of soil and foliage as a function of distance downwind from uranium mill tailings

Date

1982

Authors

Skinner, Dawn J., author
Whicker, F. Ward, advisor
Olson, H. G., committee member
Ibrahim, Shawki A., committee member

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Abstract

This study concerned 226Ra contamination of soils and foliage as a function of distance downwind from a uranium mill tailings pile. In soils the radium contamination was primarily associated with particle sizes < 0.045 mm and mainly found within the 0-0.6 cm soil horizon. The 0-0.6 cm soil horizon showed a decrease in activity concentration with distance. The 0-15 cm and 0-30 cm soil depth samples also showed a significant decrease with distance. An attempt was made using ultrasonic washing to separate internal from external 226Ra contamination in Artemisia tridentata. Internal contamination appeared to be a larger contributor to total contamination at distances ? 0.16 km downwind from the tailings pile. At distances > 0.16 km, external contamination became a larger contributor to the total 226Ra contamination. Concentration ratios (based on total contamination and internal contamination) were determined as a function of distance downwind from the tailings pile. Concentration ratios appeared to be highly site specific, however higher values (0.8-2.8) were generally associated with distances ? 0.16 km from the mill. At distances > 0.16 km. In most soil samples 226Ra concentrations approached background levels at a distance of 1.1 km from the tailings pile. Total vegetation contamination approached background at 6.6 km. A trend of decreasing internal and external 226Ra contamination with distance downwind was found to be significant (p < 5%). This study suggested that a combination of root uptake and foliar absorption were responsible for internal contamination and further studies were suggested.

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Subject

Uranium mill tailings -- Environmental aspects
Radioactive pollution of soils
Plants -- Effect of radioactive pollution on

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