Nelson, Robert Roland, authorKummerow, Christian D., advisorO'Dell, Christopher W., advisorDenning, A. Scott, committee memberPierce, Jeffrey R., committee memberHoeting, Jennifer A., committee member2019-06-142019-06-142019https://hdl.handle.net/10217/195266The scattering effects of clouds and aerosols are one of the primary sources of error when making space-based measurements of carbon dioxide. This work describes multiple investigations into optimizing how aerosols are parameterized in retrievals of the column-averaged dry-air mole fraction of carbon dioxide (XCO2) performed on near-infrared measurements of reflected sunlight from the Orbiting Carbon Observatory-2 (OCO-2). The primary goal is to enhance both the precision and accuracy of the XCO2 measurements by improving the way aerosols are handled in the NASA Atmospheric CO2 Observations from Space (ACOS) retrieval algorithm. Two studies were performed: one on using better informed aerosol priors in the retrieval and another on reducing the complexity of the aerosol parameterization. It was found that using ancillary aerosol information from the Goddard Earth Observing System Model, Version 5 (GEOS-5) resulted in a small improvement against multiple validation sources but that the improvements were restricted by the accuracy and limitations of the model. Implementing simplified aerosol parameterizations that allowed for the retrieval of fewer parameters sometimes resulted in small improvements in XCO2, but further work is needed to determine the optimal way to handle the scattering effects of clouds and aerosols in near-infrared measurements of XCO2. With several multi-million dollar space-based greenhouse gas measurement missions scheduled and in development, the massive amount of measurements will be an incredible boon to the global scientific community, but only if the precision and accuracy of the data are sufficient.born digitaldoctoral dissertationsengCopyright and other restrictions may apply. User is responsible for compliance with all applicable laws. For information about copyright law, please see https://libguides.colostate.edu/copyright.aerosol parameterizationsCO2OCO-2carbon dioxideACOSOCO2Text