Browsing by Author "Fairbank, William, advisor"
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Item Open Access Detection of small numbers of barium ions implanted in solid xenon for the EXO experiment(Colorado State University. Libraries, 2012) Cook, Shon, author; Fairbank, William, advisor; Lee, Siu Au, committee member; Roberts, Jacob, committee member; Bartels, Randy, committee memberIn an effort to discover the yet-unknown absolute masses of neutrinos, the goal of the Enriched Xenon Observatory is to observe neutrinoless double beta decay of 136Xe. Identification of this very rare decay may be difficult even with the best conventional efforts to reduce and reject radioactive background, thus requiring additional background rejection via detection of the daughter 136Ba nucleus. One method of detection is laser-induced fluorescence of the barium atom in solid xenon. Spectra of very small numbers of barium atoms in solid xenon, as few as 3 atoms, are reported for the first time. Demonstration of detection of Ba atoms with large fluorescence efficiencies gives promise for detecting single atoms in the near future. Results from experiments involving implantation of Ba+ ions in solid xenon are discussed. One narrow excitation peak was discovered from ion beam deposition that was not found in neutral deposits. Five new emission lines are found with this same excitation spectrum. Bleaching, annealing, and laser dependence of these lines are studied. The identification of the new Ba species as Ba+ or as a barium molecule is discussed.Item Open Access Imaging individual barium atoms in solid xenon by scanning of a focused laser for use in the nEXO experiment(Colorado State University. Libraries, 2019) Chambers, Christopher, author; Fairbank, William, advisor; Lee, Siu Au, committee member; Wilson, Robert J., committee member; Van Orden, Alan, committee memberNeutrinoless double beta decay (0νββ) is a non-standard model decay process in which two simultaneous beta decays occur, with no emission of neutrinos. This decay is of great interest. If observed, it will demonstrate that the neutrino and anti-neutrino are not distinct. This decay also violates lepton number conservation, a requirement for some theories seeking to explain the matter-antimatter asymmetry of the universe. A measurement of the decay half-life will also give information on the absolute mass scale of the neutrinos. EXO-200 and nEXO use liquid xenon (LXe) time projection chambers (TPC) to search for 0νββ decay. EXO-200 first observed two neutrino double beta decay (2νββ) in xenon-136, the rarest decay ever observed. A low background measurement is vital to maximizing sensitivity to the 0νββ decay mode, yet to be observed. In this dissertation, research and development of a technique for positive identification of the barium-136 daughter (barium tagging) is presented. It is desirable to incorporate barium tagging into the future nEXO detector, as it provides discrimination against all background except for the 2νββ decay mode. The scheme being developed in this work involves extraction of the barium daughter in solid xenon with a cryogenic probe, followed by matrix-isolation fluorescence spectroscopy to tag the barium atom. This work focuses on the detection of individual barium atoms in a prepared solid xenon sample. Single atom sensitivity has been achieved, and a method for imaging of individual atoms by scanning of a focused laser has been demonstrated.Item Open Access In-situ laser tagging of barium ions in liquid xenon for the EXO experiment(Colorado State University. Libraries, 2012) Hall, Kendy, author; Fairbank, William, advisor; Toki, Walter, committee member; Marconi, Mario, committee member; Roberts, Jacob, committee memberThe goal of the Enriched Xenon Observatory (EXO) collaboration is to measure the half-life of neutrino-less double beta decay using a ton size liquid 136Xe detector with zero back-ground. Zero background detection can only be achieved if the daughter nucleus, 136Ba, can be tagged. The EXO collaboration is investigating several techniques to tag the 136Ba daughter. The goal of this thesis is to investigate the prospects of directly observing a single 136Ba+ ion in the liquid using a laser aimed at the decay site, hence in-situ laser tagging. Because the energy levels of Ba+ ions are expected to be altered from the vacuum configuration, in-situ laser tagging can only be accomplished if the spectroscopy of the Ba+ ions in liquid xenon is understood. An ultra-pure liquid xenon test apparatus with a liquid xenon purity monitor has been built to study the spectroscopy of the Ba+ ions. An unexpected discovery of the nonresonant multiphoton ionization of liquid xenon using pulsed UV lasers was made while characterizing the purity monitor. The discovery was vital to the ability to accurately measure the purity of the liquid xenon. The spectroscopy of Ba+ ions in liquid xenon and the multiphoton ionization studies are the two key topics that are presented in this thesis.Item Open Access Mobility and fluorescence of barium ions in xenon gas for the EXO experiment(Colorado State University. Libraries, 2014) Benitez Medina, Julio Cesar, author; Fairbank, William, advisor; Berger, Bruce, committee member; Lundeen, Stephen, committee member; Menoni, Carmen, committee memberThe Enriched Xenon Observatory (EXO) is an experiment which aims to observe the neutrinoless double beta decay of 136Xe. The measurement of this decay would give information about the absolute neutrino mass and whether or not the neutrino is its own antiparticle. Since this is a very rare decay, the ability to reject background events by detecting the barium ion daughter from the double beta decay would be a major advantage. EXO is currently operating a detector with 200 kg of enriched liquid xenon, and there are plans to build a ton scale xenon detector. Measurements of the purity of liquid xenon in our liquid xenon test cell are reported. These results are relevant to the research on detection of single barium ions by our research group at Colorado State University. Details of the operation of the purity monitor are described. The effects of using a purifier, recirculation and laser ablation on the purity of liquid xenon are discussed. Mobility measurements of barium in xenon gas are reported for the first time. The variation of mobility with xenon gas pressure suggests that a significant fraction of molecular ions are formed when barium ions interact with xenon gas at high pressures. The measured mobility of Ba+ in Xe gas at different pressures is compared with the predicted theoretical value, and deviations are explained by a model that describes the fraction of molecular ions in Xe gas as a function of pressure. The results are useful for the analysis of experiments of fluorescence of Ba+ in xenon gas. It is also important to know the mobility of the ions in order to calculate the time they interact with an excitation laser in fluorescence experiments and in proposed 136Ba+ daughter detection schemes. This thesis presents results of detection of laser induced fluorescence of Ba+ ions in Xe gas. Measurements of the pressure broadening of the excitation spectra of Ba+ in xenon gas are presented. Nonradiative decays due to gas collisions and optical pumping affect the number of fluorescence counts detected. A model that treats the barium ion as a three level system is used to predict the total number of fluorescence counts and correct for optical pumping. A pressure broadening coefficient for Ba+ in xenon gas is extracted and limits for p-d and d-s nonradiative decay rates are extracted. Although fluorescence is reduced significantly at 5-10 atm xenon pressure, the measurements in this thesis indicate that it is still feasible to detect 136Ba+ ions directly in high pressure xenon gas, e.g. in a double beta decay detector.